For lambic I'd say the best options are BierCab, La Cerveteca (overpriced but good Belgian bottles in general) and Mikkeller Bar (I know Mikkeller's not popular here but I like their stuff and they have Cantillon, Tilquin, and 3F the majority of the time). BierCab has a ton of lambic bottles to drink there and to go, that's the place where I got a couple Armand bottles last year. No Armands on the menu when I went a few weeks ago but they had A&G, Tilquin Squared, OGV, St Lam, Hanssens Kriek, and a bunch of other good stuff.I need tips for barcelona.
Also liked the BrewDog pub but no lambic there (and it's close to Mikkeller).
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