I went and bought the same 1/10 horsepower pump you used from Freight Harbor today. Will add fittings to required hose sections and use the system on my next brew day. Har!
It's going to depend on how cold your chill water is. A larger diameter means you can flow a lot more wort but if your chill water isn't very cold, then there won't be enough heat transfer to chill that larger wort flow. You can pretty easily get 1 GPM out of 3/8" OD tubing with even a modest pump, and you will need a good flow of 60ish F (or lower) water to chill to 68 F. In a 1/2" OD tube, your flow rate can increase by about 75%. With the same chill water supply, you might find yourself metering the wort flow down to make sure the exit temp is where you want it, which negates the benefit of the larger tube for more flow.
In short, don't go larger on the wort line unless you have a adequate chill water to pull off the larger flow.