The real most critical steps are:
Recipe (no one wants to say it, but yeah)
Fermentation temp control, usually aim for the ultra low end of the yeast's temp range, or below, and support yeast growth and fermentation at that ultra low temp through pure O2 oxygenation, more than the recommended number of yeast cells to start, and ramping the temp as yeast activity slows.
For the actual all grain part, get a mill and mill your grains just before mashing. Use good water. Know your pH. Adjust your pH if it is not in the range you want it, you can use acidulated malt or lactic acid, or use RO water and build your water profile to fit your needs.
Efficiency is good, but it's not part of the best tasting all grain beer discussion. Consistency is more important so that you can make predictable adjustments from one batch to the next. This is where having your own mill is pretty important.
And if you do all that and your beer gets infected...look into your sanitation practices. And in case you, a person looking to make "the best tasting all grain beer" don't already know, you need to follow basic sanitation practices on the cold side of brewing because you have a substance that will be stored for a considerable amount of time and can develop bacterial infections if you're not careful. Not really the difference between mediocre all grain and the very best all grain at all. Mostly the difference between drinkable beer and undrinkable beer, so since drinkable beer falls into the "best tasting" beer category, yes, you do need to be sanitary.
I am with you most of the way - recipe is super-important, so are basic sanitation and temp control.
But - having your own mill? Also you don't really need to mill "just before brewing". Milled grain doesn't really go bad overnight.
Pure O2 oxygenation and pH adjustments? More than recommended yeast cells?
You can make a fantastic beers using your LHBS mill, oxygenating by 1) making a started and 2) shaking the fermenter.
You can make a starter of active, healthy yeast and pitch the recommended amount.
It's important to know your water and its weak points, but I suspect for most people just cutting the water with some RO water is sufficient to get 95% there. If you understand pH adjustments and can do them with confidence - good for you, but for the most part they can easily backfire for most people, who would struggle with even calibrating pH meter on daily basis, never mind figuring out the buffer properties of their water with some salts and acids added.
I would say freshness (or proper storage) of hops is much more important than freshness of milled grain. Simply filtering your water through carbon filter (to remove chlorine) is a major step that most brewers I know don't even do.
Once one has basic sanitation techniques (like diluting starsan in water at proper concentration and dipping/washing everything in it for 30 seconds), proper post-boil beer transfer skills are much more important than whatever gains you get from extra-sanitation efforts or worrying about trub getting into the fermenter or tiny bit of hot-side areation.
Making a fresh, active, oxygenated starter instead of repitching on a yeast cake full of dead yeast makes a lot more sense to me.
Good quality ingredients, interesting and well-designed recipes, yeast health and proper (fairly basic) tools and techniques, plus some good amount of caring, thinking and understanding the processes involved will go a long way.
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